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VOLUME 47 (1988) | ISSUE 2 | PAGE 82
Vibrational spectra of "hot" molecules in an excited electronic state: measurement of picosecond cooling kinetics by means of coherent Raman scattering
The spectra of the coherent resonant Stokes Raman scattering of trans-stilbene in an excited electronic state in a solution have been measured with picosecond time resolution/The changes in the spectra produced as a result of a photoinduced reduction of the lifetime of the Sx state reflect the kinetics of the "cooling" of the vibrational subsystem of the excited molecules.