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VOLUME 45 (1987) | ISSUE 2 | PAGE 69
Dynamics of excited electronic states of polyatomic molecules: study by picosecond coherent anti-Stokes Raman spectroscopy
The vibrational structure and dynamics of an excited electronic state of a polyatomic molecule, nickel octaethylporphyrine, have been measured at a picosecond time resolution for the first time. The experimental method was coherent anti-Stokes Raman spectroscopy. The decay time of the population of a lower-lying excited electronic state Td of this molecule in tetrahydrofuran has been determined from the kinetics of the coherent Raman spectra: 290 + 50 ps.