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VOLUME 35 (1982) | ISSUE 4 | PAGE 155
Observation of electronic predissociation of vibrationally overexcited polyatomic molecules
A new type of electronic predissociation of a polyatomic molecule has been observed for the particular case of (CF3)3CI. This predissociation results from the many-photon IR excitation of the molecule above the dissociation energy in the electronic ground state and from a mixing of the real vibrational continuum of the ground state with an unstable excited electronic state.