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VOLUME 25 (1977) | ISSUE 1 | PAGE 52
Mechanism of collisionless dissociation of molecules in the strong field of an IR laser
A new mechanism is proposed for collisionless dissociation of polyatomic molecules in a strong IR-laser field; this mechanism takes into account the possibility of cancellation of the anharmonicity of the oscillations as a result of conversion of an appreciable fraction of the vibrational energy of the molecule into rotational energy.