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VOLUME 37 (1983) | ISSUE 1 | PAGE 14
Dephasing in steady-state and time-varying spectroscopy
The Green's function h (t) describing the temporal response of a medium to a resonant field is determined for arbitrary pressures ρ and for an arbitrary dephasing correlation В (τ). The increase in the dephasing time corresponding to Dicke contraction and the identification of В (τ) from h (t) are discussed. The theory agrees with data from picosecond coherent anti-Stokes Raman spectroscopy of hydrogen at pressures in the range ρ = 10~2-10 atm.