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VOLUME 37 (1983) | ISSUE 8 | PAGE 365
Diode laser spectroscopy of SF6 molecules, cooled in a pulsed jet, with IR multiphoton excitation
The dynamics of the depletion of separate vibrational-rotational states with IR multiphoton excitation of molecules, cooled in a pulsed jet, are studied for the first time with the help of a frequency-tunable diode laser. The fraction of molecules excited by the laser pulse from separate rotational sublevels is measured and its dependence on the excitation conditions is studied.