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VOLUME 22 (1975) | ISSUE 11 | PAGE 560
Nonlinear spectroscopy based on the effect of resonant optical detection
We investigate the principles of a new type of nonlinear spectroscopy, based on the effect of resonant optical detection. It is shown that the use of one frequency-tunable light source permits measurement of the magnitude and dispersion of the nonlinear susceptibility. We discuss also a new possibility of nonlinear ultrahigh-resolution spectroscopy.