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VOLUME 28 (1978) | ISSUE 9 | PAGE 583
Spectral manifestations of various mechanisms of rotational relaxation in dense media
The transformation of the contour of the Q branch of the CARS (coherent anti-Stokes Raman Spectroscopy) spectrum in the case of strong and weak collisions is calculated. The presence of a initial-broadening stage preceding the narrowing of the spectrum is demonstrated. Methods of experimentally determining the collision forces at high densities are proposed.