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VOLUME 23 (1976) | ISSUE 4 | PAGE 217
Selectivity of dissociation of polyatomic molecules in a two-frequency IR laser field
A method is proposed for the dissociation of polyatomic molecules in a two-frequency IR laser field. In this method, a weak resonant field excites the molecules selectively, and a strong nonresonant subsequent field produces excitation into the quasicontinuum and dissociation. An appreciable increase of the dissociation selectivity is obtained.