Relaxation time mapping of single quantum dots and substrate background fluorescence
E. Pshenay-Severin+*, I. Mukhin×°, S. Fasold+, R. Geiss+, A. Steinbrck+, R. Grange+, A. Chipouline+, T. Pertsch+
+Institute of Applied Physics, Abbe Center of Photonics, Friedrich-Schiller-Universitt Jena, 07743 Jena, Germany
*Nonlinear Physics Center, Research School of Physics and Engineering, Australian National University,
ACT 0200 Canberra, Australia
×St. Petersburg Academic University, 194021 St. Petersburg, Russia
°St. Petersburg National Research University of Information Technologies, Mechanics and Optics,
197101 St. Petersburg, Russia
Abstract
We experimentally investigated the role of background signal in time resolved
photoluminescence experiments with single quantum dots on substrates. We show
that the background fluorescence signal from thin gold films fabricated by
electron-beam evaporation and from Al2O3 layers fabricated by atomic
layer deposition have to be taken into consideration in experiments on the
single photon level. Though all investigated components can be distinguished
by their photoluminescence decay rates, the presence of the background signal
prevents the observation of photon anti-bunching from single quantum dots.
Moreover, a single quantum dot acts as a hot-spot enabling the plasmon
supported fluorescence enhancement of gold.