Multigap superconductivity in iron-free pnictide BaPd2As2 revealed by local magnetization and SNS-Andreev spectroscopy
E. M. Ivanova, A. T. Daniyarkhodzhaev, L. A. Morgun, B. I. Massalimov, A. V. Sadakov, A. S. Usoltsev1)
P. N. Lebedev Physical Institute, Russian Academy of Sciences, 119991 Moscow, Russia
Abstract
We present experimental study of the iron-free palladium based analogue of the 122 iron
arsenide. Single crystals of BaPd2As2 with sharp superconducting transition were studied by two
distinct techniques: local magnetization and Break-Junction. Local magnetization was used to
obtain temperature dependence of the first critical field (Hc1) from Tc down to 10 mK. Extracted
data was fitted with various models to obtain order parameter value and draw a conclusion about
its potential symmetry. The Hc1(T) data fitting with theoretical models suggested either a single
s-wave
gap with high anisotropy factor or two s-wave gaps. Multiple Andreev Reflections
spectroscopy was used to determine the quantity of condensates and their order parameter
amplitudes. The experimental results of Multiple Andreev Reflections showed the presence of two
gap-like features. Studying Andreev spectra temperature evolution from 1.6 K up to Tc we've
extracted the gap temperature dependencies. Further fitting proved the presence of two
superconducting condensates. The obtained evidence for two gap superconductivity in iron-free
analogue of 122 iron arsenide family is reported for the first time. Despite the two gap
superconducting state, the characteristic ratio of the large gap value is almost equal to that typical
for Bardeen-Cooper-Schrieffer theory; this result shows that BaPd2As2 is a conventional
superconductor unlike BaFe2As2.